Experimentally, there is clear evidence for adsorbate / adsorbate interactions in heat of adsorption data.
2.
Thus, to optimize a MOF for carbon capture, low heat capacities and heats of adsorption are desired.
3.
In these applications, their high heat of adsorption and ability to hydrate and dehydrate while maintaining structural stability is exploited.
4.
The principle can be shown graphically by plotting the reaction rate against a property such as the heat of adsorption of the reactant by the catalyst.
5.
Rough inhomogeneous surfaces have multiple site-types available for adsorption, with some parameters varying from site to site, such as the heat of adsorption.
6.
The key assumption used in deriving the BET equation that the successive heats of adsorption for all layers except the first are equal to the heat of condensation of the adsorbate.
7.
He derived a model assuming that as the surface is loaded up with adsorbate, the heat of adsorption of all the molecules in the layer would decrease linearly with coverage due to adsorbate / adsorbate interactions:
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Where E _ 1 is the heat of adsorption for the first layer, and E _ \ mathrm { L } is that for the second and higher layers and is equal to the heat of liquefaction.
9.
It should be noted, however, that deuteration changes the heats of adsorption and the boiling and freezing points of molecules ( boiling points : 100.0 �C for H 2 O vs . 101.42 �C for D 2 O; melting points : 0.0 �C for H 2 O, 3.82 �C for D 2 O ), p " K " a ( i . e ., dissociation constant : 9.71?0 " 15 for H 2 O vs . 1.95?0 " 15 for D 2 O, cf.
10.
It should be noted, however, that deuteration changes the heats of adsorption and the boiling and freezing points of molecules ( boiling points : 100.0 �C for H 2 O vs . 101.42 �C for D 2 O; melting points : 0.0 �C for H 2 O, 3.82 �C for D 2 O ), pKa ( i . e ., dissociation constant : 9.71x10 " 15 for H 2 O vs . 1.95x10 " 15 for D 2 O, cf . heavy water ) and the strength of hydrogen bonding.
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